When an application doesn't respond, it's usually accompanied by it gobbling up system resources. Should that application consume all your remaining CPU or RAM, your system could become unresponsive, ...
The simplest and most direct way to permanently delete files or folders is by using the Shift + Delete keyboard shortcut.
I've shown you the basics of each command. When you first start using Linux, that's all you'll need. However, as you keep going, you might need to use the more advanced features of those commands. The ...